Direct Convertion Of Methane To Liquid Hydrocarbons Using HZSM-5 Zeolite Catalyst Loaded With Metal

D. D. Anggoro

doi:10.14710/reaktor.7.1.7-13

DOI: https://doi.org/10.14710/reaktor.7.1.7-13

Direct Convertion Of Methane To Liquid Hydrocarbons Using HZSM-5 Zeolite Catalyst Loaded With Metal

*D. D. Anggoro - , Indonesia

Published: 19 Jun 2017.

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Abstract

Methane is the main component of natural gas and this research provides the platrorm on the potential of utilizing natural gas, found abundant in Indonesia, to form gasoline. The objectives of the research are to modify HZSM-5 zeolite with a series of transition metals (Cr, Mn, Co, Ni, Cu, and Pt) and Ga , and to evaluate the performances of these catalyst for the single step conversion of methane to gasoline. The oxidation of methane were carried out in a micro-packed bed reactor at atmoepheric pressure, temperature 800 ⁰C, F/W = 10440 ml/g.hr and 9%vol O₂. Metals were loaded into the HZSM-5 zeolite by the wetness incipient impregnation method. The characterization results indicated that the ionic metals (Mⁿ⁺) occupy the H+ position of HZSM-5 and metal loaded HZSM-5. Ni- HZSM-5, Cu- HZSM-5 and Ga- HZSM-5 gave a high methane conversion and high gasoline selectivity. Among the catalyst samles tested, Cr- HZSM-5 showed the highest Research Octane Number (RON=86). These catalyst have the potential to convert natural gas to C₅⁺ liquid hydrocarbons provided the oxidation, dehydration and oligomerization function of the metals are in balance.

Keywords : direct conversion, methane, liquid hydrocarbons, metal, HZSM-5

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Keywords: direct conversion, methane, liquid hydrocarbons, metal, HZSM-5

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Section: Research Article

Language : ENGLISH

In Volume 07 No. 1 Juni 2003

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