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Investigation of Electrochemical, Thermal and Electrical Performance of 3D Lithium-Ion Battery Module in a High -Temperature Environment

1Department of Electrical Engineering Delhi Technological University, Delhi-110042, India

2Department of Applied Physics, Delhi Technological University, Delhi-110042, India

Received: 23 Jul 2019; Revised: 24 Apr 2020; Accepted: 30 Apr 2020; Published: 15 Jul 2020; Available online: 1 May 2020.
Editor(s): H Hadiyanto
Open Access Copyright (c) 2020 The Authors. Published by Centre of Biomass and Renewable Energy (CBIORE)
Creative Commons License This work is licensed under a Creative Commons Attribution-ShareAlike 4.0 International License.

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In the present time, the rechargeable lithium-ion battery is being commercialized to meet the sustained market’s demands. To design a more reliable, safe, and efficient Li-ion battery, a 3-D simulation study has been presented in this paper. In this study, a lithium-ion coin-cell is proposed which has LiFePO4 as a positive electrode with a thickness of 1.76 µm, carbon as a negative electrode with a thickness of 2.50 µm and Celgard 2400 polypropylene sheet as a separator between the electrodes with a thickness of 2 µm. The proposed Li-ion battery has been designed, analyzed, and optimized with the help of Multiphysics software. The simulation study has been performed to analyze the electrochemical properties such as cyclic voltammetry (CV) and impedance spectroscopy (EIS). Moreover, the electrical and thermal properties at the microscopic level are investigated and optimized in terms of surface potential distribution, the concentration of electrolyte, open circuit, and surface temperature with respect to time. It has been noticed that the peak voltage, 3.45 V is observed as the temperature distribution on the surface varies from 0 OC to 80 OC at a microscopic scale with different C-rates. The analysis of simulation results indicates a smoother electrode surface with uniform electrical and thermal properties distribution resulting in improved reliability of the battery. The performed simulation and optimization are helpful to achieve control over battery performance and safe usage without any degradation of the environment.

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Keywords: Lithium-ion battery; Electrolyte; Electrode; Current; Potential; Thermal model; Renewable Energy

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Section: Original Research Article
Language : EN
  1. Bahiraei, F., Ghalkhani, M., Fartaj, A., and Nazri, G., (2017) A pseudo-3D electrochemical-thermal modeling and analysis of a lithium-ion battery for electric vehicle thermal management applications, Applied Thermal Engineering 125, 904-918.
  2. Cai, L., and White, R., (2011) Mathematical modeling of a lithium-ion battery with thermal effects in COMSOL Inc. Multiphysics (MP) software, Journal of Power Sources 196 (14), 5985-5989.
  3. Cassagneau, T., and Fendler, J., (1998) High-density rechargeable lithium‐ion batteries self‐assembled from graphite oxide nanoplatelets and polyelectrolytes, Advanced Materials 10 (11), 877-881.<877::AID-ADMA877>3.0.CO;2-1
  4. Dai, M., Huo, C., Zhang, Q., Khan, K., Zhang, X., and Shen, C., (2018) Electrochemical Mechanism and Structure Simulation of 2D Lithium‐Ion Battery," Advanced Theory and Simulations 1 (10), 1800023.
  5. Kang, D. H.P., Chen, M., and Ogunseitan, Oladele., (2013) Potential environmental and human health impacts of rechargeable lithium batteries in electronic waste, Environmental science & technology 47 (10), 5495-5503.
  6. Hellwig, C., Sorgel, S., and Bessler, W., (2011) A multi-scale electrochemical and thermal model of a LiFePO4 battery, ECS Transactions 35 (32), 215-228
  7. Jiang, T., Zhang, S., Qiu, X., Zhu, W., and Chen, L., (2007) Preparation and characterization of silicon-based three-dimensional cellular anode for lithium-ion battery, Electrochemistry communications 9 (5), 930-934.
  8. Kukkonen, S., Erkkila, V., Manninen, A., Haavisto, J., and Pihlatie, M., (2015) Method for dimensioning battery and thermal management systems for heavy-duty vehicle applications using aged battery experimental data and advanced modeling techniques, ECS Transactions 68 (2), 83-95.
  9. Li, L., Dunn, J., Zhang, X., Gaines, L., Chen, R., Wu, F., and Amine, F., (2013) Recovery of metals from spent lithium-ion batteries with organic acids as leaching reagents and environmental assessment, Journal of Power Sources 233, 180-189.
  10. Majeau-Bettez, G., Hawkins, T., and Stromman, A (2011) Life cycle environmental assessment of lithium-ion and nickel-metal hydride batteries for plug-in hybrid and battery electric vehicles, Environmental science & technology 45 (10), 4548-4554.
  11. Notter, D., Gauch, M., Widmer, R., Wager, P., Stamp, A, Zah, R., and Althaus, H., (2010) Contribution of Li-ion batteries to the environmental impact of electric vehicles.
  12. Nyman, A., Ekstrom, H., and Fontes, E., (2012) Modeling the Lithium-ion battery," IEEE Spectrum: Technology & Science
  13. Smith, K., (2006) Electrochemical modeling, estimation, and control of lithium-ion batteries
  14. Smith, K., and Wang, C., (2006) Power and thermal characterization of a lithium-ion battery pack for hybrid-electric vehicles, Journal of power sources 160 (1), 662-673.
  15. Singh, P., Khare, N., and Chaturvedi. P, "COMSOL Modelling for Li-ion Battery Diagnostics, 2014
  16. Thanagasundram, S., Arunachala, R., Makinejad, K., Teutsch, T., and Jossen, A., 2012 (unpublished) presented at the European Electric Vehicle Congress
  17. Uddin, K., Perera, S., Widanage, W., Somerville, L., and Marco, J., (2016) Characterising lithium-ion battery degradation through the identification and tracking of electrochemical battery model parameters, Batteries 2 (2), 13.
  18. Wanger, T., (2011) The Lithium future-resources, recycling, and the environment, Conservation Letters 4 (3), 202-206.
  19. Ye, Y., Shi, Y., Cai, N., Lee, J., and He, X., (2012) Electro-thermal modeling and experimental validation for lithium-ion battery, Journal of Power Sources 199, 227-238.
  20. Zaghib, K., Charest, P., Guerfi, A., Shim, J., Perrier, M., and Striebel, K., (2005) LiFePO4 safe Li-ion polymer batteries for clean environment, Journal of power sources 146 (1-2), 380-385.
  21. Zavalis, T., Behm, M., and Lindbergh, G., (2012) Investigation of short-circuit scenarios in a lithium-ion battery cell, Journal of The Electrochemical Society 159 (6), A848-A859.

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